it seems to me that you started having problems after the flora started, you can see that it's not an excess of nutrients because it was losing color until it started to burn, and you didn't exaggerate in anything from what I think, some very clear signs of lack of calcium are those "burned" balls, unfortunately I don't have much knowledge in organic, but you will need to do a better coverage when you get into the flora, guano alone will not guarantee a good coverage